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X-ray photoelectron spectroscopy (XPS) (Fig. 4A and you can Si Appendix, Fig. S7) suggests obvious Ta and you can O trait absorption peaks, in which the clean air atoms try bonded having carbon dioxide. In addition, HAADF and effort dispersive spectrometry (EDS) mapping photos (Fig. 4B) reveal atomically spread Ta atoms. This gives all of us determination to determine if or not Ta atoms gamble a great secret role in the stage transition. To solve this issue, i created a model to replicate it changeover (Quand Appendix, Fig. S8). 4C shows that the brand new activation burden of the O-terminated program rather than tantalum atoms try 0.forty eight eV/tool phone, whilst it greatly reduces in order to −step three.99 eV/device telephone to your Ta-additional O-ended program.